Radiative lifetimes of theSandDRydberg levels of Na

Abstract
We have determined the radiative lifetimes of the n=513, s and d states of Na by pumping the desired level with two resonant photons derived from two dye lasers excited by the same N2 laser. The lifetimes increase approximately as the cube of the effective quantum number, and are in good agreement with a Coulomb-approximation calculation.