Surface-phonon dispersion in ultrathin epitaxial films of Ni on Cu(001)

Abstract
New measurements by high-resolution electron-energy-loss spectroscopy confirm the presence of localized film modes for ultrathin epitaxial films of nickel on a copper (001) substrate. These film modes, predicted recently in lattice-dynamical calculations by Chen, Wu, Yao, and Tong [Phys. Rev. B 39, 5617 (1989)] lie above the Cu-substrate bands and correspond to vibrational motion localized in the Ni overlayer. The Rayleigh-mode dispersion for the epitaxial overlayers is also reported.