Resonant multiphoton ionisation with intense monochromatic lasers

Abstract

A theoretical procedure is presented for the evaluation of resonant multiphoton ionisation rates for atoms interacting with intense monochromatic lasers. The essence of the procedure is to treat first the strong coupling by solution of the truncated Schrodinger equation to obtain a time-dependent superposition state. This is then used as the lowest order approximation to iterate the full time-dependent Schrodinger equation to obtain the transition amplitude to the continuum. A model-atom study of the time evolution of the ionisation probability is carried out and the approach to rate behaviour in the long-time limit is demonstrated. Ionisation rates are evaluated for a variety of resonant processes in H, Na and Cs involving one or two lasers, as a function of intensities and detunings. Comparison with experiment is still in a fragmentary stage, and some large discrepancies are found to exist.