Abstract
Type-II superconductors with κ1 exhibit a first-order phase transition at Hc1, which is due to an attractive interaction between flux lines. This behavior shows up as a discontinuous increase of the flux density from zero to a certain value B0. We have measured B0 as a function of temperature T, Ginzburg-Landau parameter κ, and impurity parameter α=0.882ξ0l, and have determined the critical values of these parameters below which a first-order transition occurs at Hc1. We further investigated the dependence of the parameters κ1 and κ2 on l and T, and we show that only the condition κ1(T)=12 determines the transition from type-I to type-II behavior. Comparison of our experimental results with recent theoretical treatments shows only qualitative agreement.