CARS thermometry in fuel-rich combustion zones
- 1 May 1984
- journal article
- Published by Optica Publishing Group in Applied Optics
- Vol. 23 (9), 1340-1346
- https://doi.org/10.1364/ao.23.001340
Abstract
Experimental and theoretical investigations of N2 coherent anti-Stokes Raman scattering (CARS) thermometry in laboratory ethylene–air diffusion flames have revealed significant nonresonant susceptibility effects in fuel-rich regions of the flames. The effects appear to be due to the size of the nonresonant susceptibility for typical hydrocarbon fuels and can give rise to significant temperature errors if not accounted for. An efficient theoretical algorithm for reducing spectra affected by nonresonant interference is presented and shown to give excellent agreement with experiment. It is shown that uncertainty about mixture composition or the values of nonresonant susceptibilities of individual constituents need not have a significant effect on CARS temperature measurement.This publication has 14 references indexed in Scilit:
- Collision width measurements of CO in combustion gases using a tunable diode laserJournal of Quantitative Spectroscopy and Radiative Transfer, 1981
- CARS Concentration Sensitivity With and Without Nonresonant Background SuppressionCombustion Science and Technology, 1981
- Pressure-Broadened Linewidths for N2 Coherent Anti-Stokes Raman Spectroscopy ThermometryApplied Spectroscopy, 1980
- CARS spectra of combustion gasesCombustion and Flame, 1979
- Background-free cars studies of carbon monoxide in a flameOptics Communications, 1979
- Effects of laser linewidth on coherent antiStokes Raman spectroscopyMolecular Physics, 1979
- Polarization-sensitive coherent anti-Stokes Raman spectroscopyApplied Physics Letters, 1979
- High resolution nonlinear spectroscopy. Dicke narrowing and dispersion of the third-order nonlinear susceptibility of H2 near the Q01 (1) vibrational resonanceOptics Communications, 1973
- Mesure des interactions entre ondes lumineuses dans diverses substancesJournal de Physique, 1971
- THE NONLINEAR THIRD ORDER DIELECTRIC SUSCEPTIBILITY COEFFICIENTS OF GASES AND OPTICAL THIRD HARMONIC GENERATIONApplied Physics Letters, 1967