Many-body effects in the emission spectrum of ZnTe under high-intensity photoexcitation

Abstract
At high photoexcitation levels the free-exciton emission band in ZnTe is characterized by a strong distortion which increases with the excitation intensity. The two main features are a peak shift towards lower energies and a broadening of the low-energy side of the emission band. These effects have been studied as a function of the pump wavelength by using a high-intensity tunable dye laser. The emission-peak shift is interpreted in terms of band-gap shrinkage and electron-phonon interaction. The broadening is attributed to the nonequilibrium distribution of LO phonons (hot phonons) and electrons (hot electrons).