THE FORBIDDEN I1ΣX1Σ+ ABSORPTION BANDS OF CARBON MONOXIDE

Abstract
The forbidden I1Σ–X1Σ+ transition of CO has been observed in absorption at high resolution in the vacuum ultraviolet region. As expected for a 1Σ1Σ+ transition, the bands consist of single Q branches, in which the lines of lowest J are either missing or very weak. Although the selection rule prohibiting Σ–Σ+ transitions is rigorous for dipole radiation at zero rotation, the I1Σ–X1Σ+ transition can occur for higher rotational levels because of Coriolis interaction with the A1Π state, which lies very close to the I1Σ state.Eight bands of the I–X system have been analyzed and from them the rotational and vibrational constants of the I1Σ state have been determined. Previous information on this state was based entirely on the study of perturbations in the A1Π state. The corresponding perturbations in the I1Σ state have now been observed. In addition, small "vibrational" perturbations in the ν = 4 and 5 levels (probably caused by interactions with the a3Π state) are found.