Observation of adiabatic rapid passage utilizing narrow infrared saturation resonances

Abstract
Population inversion by adiabatic rapid passage (ARP) utilizing narrow saturation resonances is observed for an infrared transition of NH3. The population change produced by sweeping the frequency of a strong saturating laser field through the center of a Doppler‐broadened absorption line is probed by a weak counterpropagating field as in a Lamb‐dip experiment. When the ARP conditions are satisfied, inversion of population is detected as amplification of the probe wave near the line center.