Abstract
The Madelung energy of the organic superconductor (2:1) tetramethylselenafulvalenium hexafluorophosphate [(TMTSF)2PF6] is −236.5798 kJ/mol (−237.3152 kJ/mol if the PF6 ion rotates freely). Its theoretical fine‐structure splitting parameters are D = 0.014 288 cm−1 and E = −0.000 557 cm−1 [nearest‐neighbor (TMTSF+)2 dimer].(AIP)

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