Depolarisation studies of positive muons in copper, vanadium, niobium and tantalum single crystals
- 1 May 1982
- journal article
- Published by IOP Publishing in Journal of Physics F: Metal Physics
- Vol. 12 (5), 875-893
- https://doi.org/10.1088/0305-4608/12/5/007
Abstract
The behaviour of positive muons ( mu +) has been studied in Cu, V, Nb and Ta single crystals, using the muon spin rotation ( mu SR) technique. The measurements were performed in the temperature regime 5-365K, in transverse external magnetic fields of 50-5500 G. In FCC Cu the mu + diffusional motion can be described in terms of quantum mechanical jump processes of a small polaron among octahedral interstitial sites. An orientation average leads to an activation energy of E=79.2+or-3.1 meV, a pre-exponential factor of D(0)=(1.66+or-0.33)*10-8 cm2 s-1 and a tunnelling matrix element of J=(18.3+or-1.8)*10-6 eV. The mu + total volume expansion was found to be Delta V=3.91 AA3. Furthermore, the electric field gradient (EFG) at the mu + nearest-neighbour nuclei has been determined as q=0.30 AA-3. In BCC V, Nb and Ta the mu + diffusion is trap-limited. As a function of the temperature the mu + probe different classes of trapping sites associated with host metal impurities. At low temperature, before decaying, the mu + always end up in a trapped state which shows that the intrinsic mu + motion between traps is fast and seems to reflect properties of a band diffusion.Keywords
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