Abstract
The generation of second-harmonic ultrasound (5 to 10 MHz) with an estimated conversion efficiency ≳ 20% has been observed for the soft shear mode in V3Si below 77°K. The harmonic generation is a manifestation of the unusually large shear anharmonicity for this unstable compound; however, static symmetry arguments forbid the generation of an even-ordered harmonic for a high-symmetry shear wave in a cubic crystal. Several possible sources of symmetry reduction are discussed.