Stratospheric Sulfuric Acid Layer: Evidence for an Anthropogenic Component

Abstract
Recent measurements of small aerosol particles in the stratosphere over Laramie, Wyoming, indicate low-concentration background conditions. A comparison of measurements made some 20 years ago with the present background concentration reveals the possibility of an increase of 9 percent per year. Since the aerosol particles are predominantly sulfuric acid droplets which form in the stratosphere from tropospheric sulfur-containing gases, such an increase may be related to man-made sulfur emissions.