Solution Dimerization of the Tetracyanoquinodimethane Ion Radical

Abstract
The reversible dimerization of the anion radical of 7,7,8,8‐tetracyanoquinodimethane in aqueous solution has been studied spectroscopically. Analysis of the spectra yields an equilibrium constant for dimerization (2A⇆A2=) at 25° of 2.5×103 liter/mole and a heat of dimerization of −10.4 kcal/mole dimer.

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