Laser Excitation of the Muonium1S2STransition

Abstract
We present evidence for the excitation of the two-photon Doppler-free 1S2S transition in muonium. Thermal muonium atoms were produced in vacuum by a 27.5-MeV/c pulsed positive-muon beam incident on a powdered SiO2 target. Transitions were induced by the light from a frequency-doubled pulsed dye laser and were detected by photoionization of the 2S state. The 1S(F=1)2S(F=1) transition frequency is within 300 MHz of the QED prediction.