Field studies were conducted in Prince Edward Island (PEI) on the Fe nutrition of cereals and forages and to determine the relationship between plant Fe and soil pH. The Fe concentration in barley (Hordeum vulgare L.) and oats (Avena sativa L.) boot stage tissue (BST) and grain ranged from 35 to 65 and from 19 to 42 mg kg−1, respectively, in the control and from 38 to 57 and from 22 to 45 mg kg−1, respectively, in the soil applied Fe treatments. In the foliar applied Fe treatments, the cereal BST contained as much as 121 mg Fe kg−1 in the FeSO4.7H2O treatments and up to 86 mg kg−1 in the chelate-Fe treatment, but neither of these two sources increased Fe concentration in the grain. In the first cut of forages in the foliar treatments, the Fe was as high as 131 mg Fe kg−1, but no differences were generally found between the control and Fe treatments in the second cut. Over the soil pH ranges of 4.5–6.9, no consistency was found in the correlation coefficient (r) values between plant Fe and soil pH. In spite of the Fe concentrations as low as 19 mg kg−1 in cereal grain and 23 mg kg−1 in forages in the control treatments, no yield response to added Fe was found. However, the Fe concentrations as found in this study would be considered deficient for livestock and mineral supplements of Fe to the feeds may be desirable. Key words: Cereals, forages, soil pH, plant iron, acid soils