Stable atmospheric methane in the 2000s: key-role of emissions from natural wetlands
Preprint
- 4 April 2013
- preprint
- Published by Copernicus GmbH in EGUsphere
Abstract
Two atmospheric inversions (one fine-resolved and one process-discriminating) and a process-based model for land surface exchanges are brought together to analyze the variations of methane emissions from 1990 to 2009. A focus is put on the role of natural wetlands and on the years 2000–2006, a period of stable atmospheric concentrations. From 1990 to 2000, the two inversions agree on the time-phasing of global emission anomalies. The process-discriminating inversion further indicates that wetlands dominate the time-variability of methane emissions with 90% of the total variability. Top-down and bottom-up methods are qualitatively in good agreement regarding the global emission anomalies. The contribution of tropical wetlands on these anomalies is found to be large, especially during the post-Pinatubo years (global negative anomalies with minima between −41 and −19 Tg y−1 in 1992) and during the alternate 1997–1998 el-Niño/1998–1999 la-Niña (maximal anomalies in tropical regions between +16 and +22 Tg y−1 for the inversions and anomalies due to tropical wetlands between +12 and +17 Tg y−1 for the process-based model). Between 2000 and 2006, during the stagnation of methane concentrations in the atmosphere, total methane emissions found by the two inversions on the one hand and wetland emissions found by the process-discriminating-inversion and the process model on the other hand are not fully consistent. A regional analysis shows that differences in the trend of tropical South American wetland emissions in the Amazon region are mostly responsible for these discrepancies. A negative trend (−3.9 ± 1.3 Tg y−1) is inferred by the process-discriminating inversion whereas a positive trend (+1.3 ± 0.3 Tg y−1) is found by the process model. Since a positive trend is consistent with satellite-derived extent of inundated areas, this inconsistency points at the difficulty for atmospheric inversions using surface observations to properly constrain tropical regions with few available observations. A consequence is the need to revisit the large increase in anthropogenic emissions computed at the global scale by some inventories for the early 2000s, although process-based models have also their own caveats and may not take into account all processes.Keywords
All Related Versions
- Published version: Atmospheric Chemistry and Physics, 13 (23), 11609.
This publication has 73 references indexed in Scilit:
- Analysis of global methane changes after the 1991 Pinatubo volcanic eruptionAtmospheric Chemistry and Physics, 2013
- Recent decreases in fossil-fuel emissions of ethane and methane derived from firn airNature, 2011
- Source attribution of the changes in atmospheric methane for 2006–2008Atmospheric Chemistry and Physics, 2011
- Large-Scale Controls of Methanogenesis Inferred from Methane and Gravity Spaceborne DataScience, 2010
- Inverse modeling of global and regional CH4 emissions using SCIAMACHY satellite retrievalsJournal of Geophysical Research: Atmospheres, 2009
- Atmospheric methane in the Mediterranean: Analysis of measurements at the island of Lampedusa during 1995–2005Atmospheric Environment, 2007
- Contribution of anthropogenic and natural sources to atmospheric methane variabilityNature, 2006
- Estimation of atmospheric methane emissions between 1996 and 2001 using a three‐dimensional global chemical transport modelJournal of Geophysical Research: Atmospheres, 2006
- Two decades of OH variability as inferred by an inversion of atmospheric transport and chemistry of methyl chloroformAtmospheric Chemistry and Physics, 2005
- Trace gas variations at Cape Point, South Africa, during May 1997 following a regional biomass burning episodeAtmospheric Environment, 2000