Ultrasonic investigation of critical dynamics in KMnF3

Abstract
An extensive ultrasonic investigation of the cubic-tetragonal phase transition in KMnF3 with respect to temperature, frequency, mode, and sample dependence has been carried out by means of wave-vector-reversed echo technique as well as conventional pulse reflections. All measurements of the attenuation α obey a dynamic scaling law αω2tρG(ωτ). We have measured ρ=1.87±0.05, in accord with the predictions of the three-dimensional Heisenberg model, a result which is consistent with the expected value φ1.26 for the anisotropy cross-over exponent. The relaxation time τ, governing the dynamics of ordered clusters, is found to be (9×1013)t1.41 s. The form of the scaling function G is experimentally determined, and its expected limiting forms at low and high ωτ values discussed.