Resonance Fluorescence and Resonance Raman Scattering: Lifetimes in Molecular Iodine
- 4 February 1974
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 32 (5), 196-199
- https://doi.org/10.1103/physrevlett.32.196
Abstract
We report a significantly shortened scattering lifetime in molecular iodine when the frequency of a single-mode 5145-ÅA incident laser is tuned away from resonance with a discrete transition. This observation of a shortened scattering time is indicative of what has been conventionally called a Raman process. Off-resonance lifetime measurements, as reported here, may provide a means of determining the relative contribution to the absorption linewidth of homogeneous and inhomogeneous broadening.Keywords
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