O18Excitation Energies and Lifetimes from Ge(Li) Measurements in theF19(t, αγ)O18Reaction

Abstract
Ge(Li) spectrometry has been used to study the γ-ray deexcitation of states of O18 produced in the F19(t, α)O*18 reaction at Et=2.6 MeV. Precision excitation energies were determined from both singles and coincidence measurements. Multiparameter data collection techniques were used to store γ-ray spectra measured at θγ=0, 45, and 90° in coincidence with α groups populating various final states of O18. α particles were detected in an annular detector at θ¯α=180°, thus defining a narrow cone of forward-going O18 recoils which stopped in the Ni target backings. The observed Doppler shifts were analyzed, via the Doppler-shift attenuation method, to determine the lifetimes of the initial γ-emitting states. Resulting excitation energies (in keV) and meanlives (in psec) for the first 15 excited states of O18 are as follows: 1982.16 ± 0.20 (τ=2.90.6+0.9), 3555.07 ± 0.45 (> 4.0), 3634.50 ± 0.40 (1.33 ± 0.20), 3920.6 ± 0.4 (0.024 ± 0.010), 4456.1 ± 0.5 (0.065 ± 0.015), 5098.5 ± 1.2 (0.062 ± 0.025), 5260.4 ± 1.2 (0.12 ± 0.03), 5336.4 ± 0.6 (0.20 ± 0.04), 5377.8 ± 1.2 (γ transition were fitted, as a function of θγ, in order to determine relative intensities and thus branching ratios. An analysis of the correlation data provides confirmation or support for previously reported conclusions on spin-parity assignments, and in addition restricts possible assignments for the 6351-keV state to J=1 or 2. These results are compared to previous data on O18 and to theoretical considerations.