Synthesis of unsymmetrical tetrathiafulvalenes and electrical conductivities of their tetracyanoquinodimethane complexes

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Abstract
The preparation of some unsymmetrical tetrathiafulvalenes and the electrical conductivities of their charge transfer complexes with tetracyanoquinodimethane (TCNQ) are described; the ethylenedithio(trimethylene)tetrathiafulvalene–TCNQ complex exhibited higher conductivity than complexes of tetrathiafulvalene, tetramethyltetrathia-fulvalene, and hexamethylenetetrathiafulvalene with TCNQ.