Interface Tension-Induced Synthesis of Monodispersed Mesoporous Carbon Hemispheres

Abstract
Here we report a novel interface tension-induced shrinkage approach to realize the synthesis of monodispersed asymmetrical mesoporous carbon nanohemispheres. We demonstrate that the products exhibit very uniform hemispherical morphology (130 × 60 nm) and are full of ordered mesopores, endowing them high surface areas and uniform pore sizes. These monodispersed mesoporous carbon hemispheres display excellent dispersibility in water for a long period without any aggregation. Moreover, a brand new feature of the mesoporous carbon materials has been observed for the first time: these monodispersed mesoporous carbon hemispheres show excellent thermal generation property under a NIR irradiation.
Funding Information
  • Ministry of Science and Technology of the People's Republic of China (2012CB224805, 2013CB934104)
  • Science and Technology Commission of Shanghai Municipality (14JC1400700)
  • National Natural Science Foundation of China (21210004, 21322311)