Effect of Imprisonment of Radiation in Sodium Vapor on the Measured Lifetime of the3 P2States

Abstract

The effect of imprisonment of radiation in sodium vapor on the measured lifetime of the $3 {}_{}{}^2{}_{}{}^{}P$ states has been investigated in an experiment in which the atoms in the vapor were excited with 10-nsec pulses of resonance radiation and the elapsed times between the exciting and the fluorescent pulses were recorded using a time-to-amplitude converter and kicksorter. At vapor densities below ${10}^{10}$ atoms/${\mathrm{cm}}^3$, where there is no multiple scattering, the measured lifetime reaches a constant value of (1.63±0.04)×${10}^{-8\mathrm{}}$ sec, equal to the natural lifetime of the $3 {}_{}{}^2{}_{}{}^{}P$ states. In the density range ${10}^9$-${10}^{13}$ atoms/${\mathrm{cm}}^3$, the variation of the effective lifetime with the vapor density is in good agreement with the predictions of Milne's theory of radiation trapping; agreement with Holstein's theory is observed only in the range ${10}^{12}$-${10}^{13}$ atoms/${\mathrm{cm}}^3$. The results of a subsidiary Hanle experiment show that a multiply scattered photon of sodium resonance fluorescence loses its original polarization and that, at high sodium vapor pressure, coherence is not preserved.