Interaction-induced effects in the nonlinear coherent response of quantum-well excitons

Abstract

Interaction-induced processes are studied using the third-order nonlinear polarization created in polarization-dependent four-wave-mixing experiments (FWM) on a ZnSe single quantum well. We discuss their influence by a comparison of the experimental FWM with calculations based on extended optical Bloch equations including local-field effects, excitation-induced dephasing, and biexciton formation. The investigations show that, for copolarized input fields, excitation-induced dephasing is the dominant FWM mechanism, followed by the conventional density-grating FWM process, biexcitonic contributions, and local-field effects. For cross-linear polarized input fields the excitation-induced dephasing mechanism is canceled so that the conventional density-grating FWM process and biexcitonic contributions are dominating.