Light scattering in Heisenberg paramagnets

Abstract
Two-spin light scattering in the disordered phase of Heisenberg antiferromagnets is investigated by means of a modified Markoffian approximation for the continued-fraction representation of the shape function. The necessary frequency moments are evaluated: they are found to be dominated by the contribution of zone-boundary wave vectors. The predicted spectral shapes are in good agreement with the experimental spectra in RbMnF3 and KNiF3 both at high temperatures and in the neighborhood of the Néel point.